Growth environment dependent phase propagation of ilmenite-hematite (1-x)FeTiO<sub>3</sub>-xFe<sub>2</sub>O<sub>3</sub> films

  • Lee, Dooyong
  • Song, Sehwan
  • Kim, Hyeonyu
  • Lee, Hyunkyung
  • Lee, Jisung
  • ... Yoon, Sangmoon
  • 외 9명
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초록

We investigated crystal structures, charge ordering, and magnetic properties of ilmenite-hematite (IH) (1-x) FeTiO3-xFe(2)O(3) films grown at various temperatures and oxygen flow rates. The IH solid solution films grown below 650 degrees C without O-2 have weak magnetic moments due to the Fe2+ in the FeTiO3 phase and Fe3+ in the alpha-Fe2O3. The film grown at 650 degrees C without O-2 exhibits the Neel temperature of similar to 60 K and a large magnetic moment due to the Fe2+ ions, resulting from an ordered FeTiO3 phase. Furthermore, the films grown at 650 degrees C under the O-2 have an alpha-Fe2O3 phase separated from FeTiO3 due to excessive O-2 during growth. As a result, the film has weak magnetic moments attributed to Fe3+ in the alpha-Fe2O3 phase. These observations show that the crystal phase and charge ordering are sensitive to the amount of O-2 and responsible for magnetic properties in the ilmenite-hematite system.

키워드

Ilmenite-hematiteSolid solutionOrder-disorder structureCharge orderingX-ray magnetic circular dichroismFETIO3DIFFRACTIONMAGNETISMSYSTEMSTATESTI
제목
Growth environment dependent phase propagation of ilmenite-hematite (1-x)FeTiO<sub>3</sub>-xFe<sub>2</sub>O<sub>3</sub> films
저자
Lee, DooyongSong, SehwanKim, HyeonyuLee, HyunkyungLee, JisungKim, MinjaeLee, JinbaeHwang, Sang WoonYoon, SangmoonKim, YounghakCho, Chang-wooJo, YounjungOk, Jong MokChung, Jae-HoPark, Sungkyun
DOI
10.1016/j.jallcom.2025.178997
발행일
2025-02
유형
Article
저널명
Journal of Alloys and Compounds
1017